Lithium-ion batteries (LIBs), while dominant in energy storage due to high energy density and cycling stability, suffer from severe capacity decay, rate capability degradation, and lithium dendrite formation under low-temperature (LT) operation. Therefore, a more comprehensive and systematic understanding of LIB behavior at LT is urgently required.
Provided by the Springer Nature SharedIt content-sharing initiative Operating aqueous redox flow batteries (ARFBs) at low temperatures is prohibited by limited solubility of redox-active materials, freezing electrolytes and sluggish reaction kinetics.
The low-temperature operating range of the battery is primarily limited by the liquid phase window of electrolytes. Due to the high melting point of commonly used carbonate solvents, the electrolyte solidifies below certain temperatures. The phase states of typical carbonate electrolytes are listed in Table 1 .
Various factors such as electrolyte viscosity, desolvation, interphase chemistry, electrode material and thickness have impact on the low-temperature performance of the battery, and these factors depend on the battery design [30, 34].
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